Now I'm listening to this.
Most of Hank's "soundtrack" albums from the 60s were re-recordings, and focused on the pop/lounge/jazz aspects of the scores rather than the dramatic music.
Sadly, as a result, Hank picked up a reputation as more a of tunesmith than anything else.
"Wait Until Dark" features the actual soundtrack recordings, and has it all - the dark moody stuff, jazz, bossa nova, everything you would hear in an insanely groovy/disturbing soundtrack of the era.
What a guy.